“Jesus Was a Crossmaker” by the Hollies
I can’t claim to have really noticed this song in Cameron Crowe’s Elizabethtown, which is where all those clips in the video come from, and on whose soundtrack this song appears. But I’m a big fan of Rachael Yamagata, and of her cover.
Actually, it’s possible her version is the one that appeared in the film and I never noticed it either. It’s on volume 2 of the soundtrack. (You can fault Crowe for a lot with that movie, but the man knows how to put together soundtracks.) It’s possible. I don’t quite feel like watching Elizabethtown again to find out.